To some degree the answer depends on whether with weight loss you retain volume in the face or not. This has a genetic determination and some people simply don't lose volume in the face even if their weight decreases. In generic terms, weight loss can help with increasing the definition of the face.Other methods that can help increase the definition include liposuction around the lower part of the cheeks, jaw line and under the chin, possibly combined with buccal fat reduction.Both your photographs are taken smiling and it is difficult to know whether the cheek volume is full or average when your faces is relaxed. Reducing the cheekbone width is generally carried out better by a reduction of bone support. I would consider it a last resort plan Computer imaging in 3D and simulation can help you understand the degree of change you wish to achieve and can qualify the type of surgery that may be suitable to assist.